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Photocatalytic water reduction with copper-based photosensitizers: a noble-metal-free system

Luo, Shu-Ping and Mejía, Esteban and Friedrich, Aleksej and Pazidis, Alexandra and Junge, Henrik and Surkus, Annette-Enrica and Jackstell, Ralf and Denurra, Stefania and Gladiali, Serafino Gabriele and Lochbrunner, Stefan and Beller, Matthias (2013) Photocatalytic water reduction with copper-based photosensitizers: a noble-metal-free system. Angewandte Chemie. International Edition, Vol. 52 (1), p. 419-423. eISSN 1521-3773. Article.

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DOI: 10.1002/anie.201205915

Abstract

Of noble descent: A fully noble-metal-free system for the photocatalytic reduction of water at room temperature has been developed. This system consists of CuI complexes as photosensitizers and [Fe3(CO)12] as the water reduction catalyst. The novel Cu-based photosensitizers are relatively inexpensive, readily available from commercial sources and stable to ambient conditions, thus making them an attractive alternative to the widely used noble-metal based systems.

Item Type:Article
ID Code:8120
Status:Published
Refereed:Yes
Uncontrolled Keywords:Copper, hydrogen, photochemistry, sustainable chemistry, water splitting
Subjects:Area 03 - Scienze chimiche > CHIM/04 Chimica industriale
Divisions:001 Università di Sassari > 01-a Nuovi Dipartimenti dal 2012 > Chimica e Farmacia
Publisher:Wiley
eISSN:1521-3773
Deposited On:08 Nov 2012 12:17

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