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Iron-catalyzed amidation of aldehydes with N-chloroamines

Porcheddu, Andrea and De Luca, Lidia Vera Giovanna (2012) Iron-catalyzed amidation of aldehydes with N-chloroamines. Advanced Synthesis & Catalysis, Vol. 354 (16), p. 2949-2953. eISSN 1615-4169. Article.

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DOI: 10.1002/adsc.201200659

Abstract

A new direct conversion of aldehydes to amides has been realized, in the presence of iron(III) chloride as a catalyst and using tert-butyl hydroperoxide (TBHP) as an oxidant. Both aliphatic and aromatic aldehydes were successfully reacted with variously mono- and di-substituted N-chloroamines. The methodology has a wide substrate scope, uses cheap and easily available reagents and is characterized by short reaction times.

Item Type:Article
ID Code:8115
Status:Published
Refereed:Yes
Uncontrolled Keywords:Aldehydes, amides, iron, radical reactions
Subjects:Area 03 - Scienze chimiche > CHIM/06 Chimica organica
Divisions:001 Università di Sassari > 01-a Nuovi Dipartimenti dal 2012 > Chimica e Farmacia
Publisher:Wiley
eISSN:1615-4169
Deposited On:07 Nov 2012 16:46

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